Single-frequency distributed Bragg reflector Tm:YAG ceramic derived all-glass fiber laser at 1.95μm

Guo-Quan Qian(錢國權(quán)) Min-Bo Wu(吳敏波) Guo-Wu Tang(唐國武) Min Sun(孫敏)Dong-Dan Chen(陳東丹) Zhi-Bin Zhang(張志斌) Hui Luo(羅輝) and Qi Qian(錢奇)

1Yunnan Police College,Kunming 650223,China

2Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques,South China University of Technology,Guangzhou 510640,China

3School of Physics and Optoelectronic Engineering,Guangdong University of Technology,Guangzhou 510006,China

4Southwest Institute of Technical Physics,Chengdu 610041,China

Keywords: all-glass fiber,single-frequency,2μm fiber laser,Tm:YAG ceramic derived

1. Introduction

Single-frequency fiber lasers operating at～2 μm have attracted intense attention for their wide-ranging applications,from high-resolution spectroscopy and noninvasive medicine to coherent beam combining,due to their outstanding properties of low noise, narrow linewidth and at an eye-safe wavelength regime.[1–4]Up to now,～2μm single-frequency fiber lasers have been achieved in various cavity structures,including ring cavities,distributed feedback(DFB)cavities and distributed Bragg reflector (DBR) cavities.[5–7]More recently,Walasiket al.reported a 2μm single-frequency all-fiber DFB laser source employing fiber Bragg gratings(FBGs)which has a laser linewidth of 5 kHz.[8]Here, we focus on a～2 μm single-frequency fiber laser with a DBR cavity structure. A key factor in obtaining a DBR single-frequency fiber laser is the use of high-gain glass fibers for shorting the laser cavity.[9]It is known that a high rare earth(RE)ion doping concentration can achieve a large pump absorption and high gain per unit length in the resulting glass fiber, which allows efficient laser output in a short piece of RE ion-doped active fiber.[10,11]

To date, single-frequency DBR fiber lasers at～2 μm have been developed by using different Tm3+-doped glass fibers, such as silica, silicate and germanate glass fibers.[7,12,13]However,pure silica glass fibers have a low RE ion doping concentration because of the well-defined glass structure consisting of a [SiO4] tetrahedron, which limits the gain of the resulting silica glass fibers.[14]In 2015, Fuet al.demonstrated a 2μm single-frequency DBR fiber laser based on a 1.9-cm long commercially available Tm3+-doped silica glass fiber; this had a maximum output power of 18 mW and a slope efficiency of 13.4% with respect to the absorbed pump of a 793 nm laser diode (LD).[7]The output power of a 2 μm single-frequency DBR fiber laser can be improved by means of in-band pumping at the 1.5 μm band.[15]Note that multicomponent glasses,which have high RE ion solubility, are usually used to fabricate high-gain glass fibers.[1,16]Genget al.reported a single-frequency DBR fiber laser at 1893 nm based on a 2 cm long heavily Tm3+-doped germanate glass fiber; this had a pump threshold of 30 mW and a maximum output power of 50 mW.[17]They went on to demonstrate a narrow-linewidth single-frequency DBR fiber laser at 1.95μm with a 2 cm long heavily Tm3+-doped silicate glass fiber.[12]However, the large splicing losses (～2.2 dB) between the active fiber and two FBGs resulted in a relatively high threshold.[12,15]In 2018, Tanget al.fabricated a heavily Tm3+-doped barium gallo-germanate glass fiber that had a gain per unit length of 3.6 dB·cm?1at 1.95μm.[13]A singlefrequency DBR fiber laser of over 220 mW at 1.95μm was realized in a 1.5 cm long active fiber,showing a slope efficiency of 30.2% with respect to the absorbed pump of a 1568 nm fiber laser.[13]Although the multicomponent glass fibers used in these reports possess higher RE ion solubility over the silica fiber,which enables～2μm single-frequency DBR fiber laser operation with higher output power and slope efficiency,there are still some obstacles to their application in the aforementioned areas.[15,18]For example, their softening temperature and thermal expansion coefficient are different from those of commercial silica glass fiber,implying that it is more challenging to achieve low-loss spliced with silica-based fiber devices,such as wavelength division multiplexer(WDM)and FBG.[7]Moreover,the resulting splice joint exhibits reduced mechanical strength, which sacrifices the reliability of the fiber laser system.[15]Therefore, the development of novel fiber materials, fiber design and fabrication techniques could facilitate some high RE ion-doped silica-based fibers becoming competitive candidates for single-frequency fiber lasers.

In recent years, RE ion-doped Y3Al5O12(YAG) single crystal or polycrystalline ceramic (precursor phase) derived all-glass fibers with novel properties have been developed and fabricated for high-power fiber lasers,ultrafast fiber lasers and single-frequency fiber lasers.[19–22]Compared with RE ion-doped silica glass fibers,YAG-derived all-glass fibers with a high yttrium (Y) and aluminum (Al) concentration in the fiber core [yttrium aluminosilicate (YAS) glass] have a higher thermal conductivity and a higher stimulated Brillouin scattering threshold, properties which are beneficial for achieving high-power single-frequency fiber lasers.[23–26]Additionally, in contrast to RE ion-doped multicomponent glass fiber, the thermal expansion coefficient and refractive index of these YAG-derived all-glass fibers better matches with the silica glass cladding, making them easier to splice with silica fibers.[22,27,28]In 2019, Zhanget al.demonstrated a singlefrequency DBR fiber laser at 1.064 μm based on a 1.7 cm long Yb:YAG ceramic-derived all-glass fiber.[19]Although the output power and slope efficiency of the laser were relatively low, this work was the first to provide a prospect for the development of all-fiber single-frequency DBR fiber lasers by using YAG-derived all-glass fibers. Then, Liuet al.reported a 110 mW single-frequency DBR fiber laser at 1.064 μm with a slope efficiency of 18.5% based on a 1.4 cm long Yb:YAG crystal-derived all-glass fiber by reducing the resonance loss.[20]More recently,Xieet al.reported a 24.2 mW pulsed single-frequency laser at 1.55 μm based on a 1.8 cm long Er:YAG crystal-derived all-glass fiber.[29]However, single-frequency DBR fiber lasers at～2 μm based on Tm:YAG crystal or ceramic-derived all-glass fibers have never been reported.

Here,Tm:YAG ceramic-derived all-glass fiber was drawn by using the molten core method. It has a gain per unit length of 2.7 dB·cm?1at 1.95 μm. The as-drawn fiber has a YAS glass core, which is composed of 14.2 mol.% Al2O3,77.1 mol.%SiO2, 6.5 mol.%Y2O3, and 2.25 mol.%Tm2O3.Details of the as-drawn YAS glass fiber can be found in Table 1. A 1.95 μm single-frequency DBR fiber laser was achieved by using a 2 cm long Tm:YAG ceramic-derived all-glass fiber. The fiber laser has a high optical signal-tonoise ratio (OSNR) of～77 dB and a low pump threshold of～15.4 mW. The direct output power of the laser reached 135 mW with a pump power of 1340 mW, corresponding to a slope efficiency of 10.2% with respect to the absorbed pump power. In addition, the linewidth and relative intensity noise(RIN)were measured. This work is a proof-of-concept that Tm:YAG-derived all-glass fiber with a high gain per unit length can be used in a compact 2μm single-frequency DBR fiber laser.

Table 1. Properties of Tm:YAG ceramic-derived all-glass fiber.

2. Experimental details

Tm:YAG ceramic samples were prepared by the solidstate reaction method. Commercial powders (Al2O3, Y2O3,Tm2O3) were weighed and then mixed. Boric acid (1 wt%)was used as a sintering aid in the samples. Column-shaped YAG ceramic samples were prepared after the pressed green bodies were sintered at 1600?C for 5 h in a muffle furnace,and then ground and polished into cylindrical rods with a diameter of～2.8 mm. The YAG rods were washed repeatedly with dilute hydrochloric acid, alcohol and distilled water to remove the contaminated surface layer and then placed into a vacuum drying oven at 400?C for 12 h. After preparation the initial precursor material was inserted into cylindrical silica glass tubes (optical quality 99.99%, inner diameter～3 mm,external diameter～30 mm,length～150 mm). One end of the tube was sealed using an oxyhydrogen flame. Optical fiber was prepared using a standard fiber drawing tower at a temperature of～2000?C.During the drawing process of the molten core method, the glass cladding is similar to‘the crucible’, which provides a high-temperature, high-pressure environment for the core material,and the molten core is rapidly quenched. Glass fibers with different diameters can be obtained by controlling the feeding speed, the temperature and the pulling speed. Hundreds of meters of fibers with an outer diameter of～125μm were collected for test characterization and laser experiments.

Figure 1(a) shows the XRD pattern of the Tm:YAG ceramic sample. The diffraction peaks of the sample match well with the standard card of YAG (PDF#33-0044), suggesting that the prepared ceramic sample is pure YAG phase. Figure 1(b) shows the Raman spectra of the resulting Tm:YAS fiber core and silica glass cladding. The broad Raman bands in the fiber core and cladding indicate the amorphous state of the obtained fiber.

Figure 2(a) shows the electron micrograph image of the Tm:YAS all-glass fiber. It can be observed that the fiber core has a good circularity. Figures 2(b)–2(e) show the electron probe microanalyzer mapping of Si, Y Al, and Tm. The Al,Tm, and Y are mainly distributed in the core region, while the Si is distributed in both the cladding and the core. In our previous work this type of YAS glass fiber was proven to be a graded refractive index fiber due to the elemental migration between the melting core and the softened cladding.[27]

Fig.1.(a)XRD pattern of the Tm:YAG ceramic sample.(b)Raman spectra of the resulting Tm:YAS glass fiber core and the silica glass cladding.

Fig.2. (a)Electron micrograph image of the Tm:YAS all-glass fiber. (b)–(e)Electron probe microanalyzer images of the distribution of different elements across the fiber cross section.

The scheme of the experimental setup for the 1.95 μm single-frequency DBR fiber laser is shown in Fig.3. The laser cavity combines a partial-reflection fiber Bragg grating (PRFBG), a high-reflection fiber Bragg grating (HR-FBG) and a short piece of as-drawn gain fiber. The two ends of the gain fiber were spliced with the PR-FBG and HR-FBG. The PRFBG has a reflectivity of 50.0%at 1950 nm and a 3 dB bandwidth of 0.09 nm. The HR-FBG has a reflectivity of 99.5%at 1950 nm. A backward pumping scheme was used in the laser experiment. The fiber laser was counter-pumped by a highpower 1610 nm fiber laser, through a 1610/1950 nm WDM.The whole laser cavity was placed in an aluminum tube,which was temperature-controlled by a cooling system with an accuracy of±0.1?C. To achieve efficient single-frequency laser operation,a short cavity length is necessary to enlarge the longitudinal mode spacing. For this purpose, a section of 2 cm long Tm:YAG-derived all-glass fiber was chosen as the gain fiber by the cut-back method. The laser output spectrum was monitored by an optical spectrum analyzer (AQ6375, Yokogawa, Japan) with a wavelength resolution of 0.02 nm. The single-frequency operation of the laser was confirmed by using a scanning fiber Fabry–Perot interferometer (FFPI; SA200-18B, Thorlabs) with a free-spectral range (FSR) of 1.5 GHz and a resolution of 7.5 MHz. The laser linewidth was measured by a self-heterodyne method. The RIN of the fiber laser was measured by an electrical spectrum analyzer,whose resolution bandwidth was set to 1 kHz. During each measurement of RIN the laser power was attenuated to 0.5 mW before being injected into a photoelectric detector.

Fig.3. Scheme of the experimental setup for the 1.95μm single-frequency DBR fiber laser based on the as-drawn gain fiber(GF).

3. Results and discussion

The laser output spectrum is shown in Fig. 4(a). The achieved laser has a central wavelength of 1950 nm with an OSNR of～77 dB. The laser output power and the residual power were measured by a standard power meter. Figure 4(b) shows the laser output power as a function of the absorbed pump power. The laser threshold was measured to be～15.4 mW. The fiber laser yields a maximum laser output power of 135 mW with a slope efficiency of 10.2%. Note that the phenomenon of power saturation was not observed,suggesting that the output power could be further improved by using a higher available pump power. The stability of the laser output power at 60 mW was measured for 40 min; the result is shown in the inset of Fig.4(b). The constructed fiber laser is stable with an output power fluctuation relative to the average power of～3.24%(relative standard deviation)during the entire period.

The scanning spectrum over the FSR of the FFPI is presented in Fig.5.A stable single-longitudinal-mode output was achieved when the temperature of the laser cavity was controlled at 19.6?C. Through the strict temperature control of the whole laser cavity, the laser operated stably in a singlefrequency regime without mode hopping or mode competition as the pump power increased. Therefore, a 135 mW singlefrequency DBR fiber laser operating at 1.95μm was realized in a 2 cm long gain fiber when in-band pumped by a 1610 nm fiber laser.

Fig.4. (a)Measured output spectrum of the fiber laser. (b)The laser output power versus the absorbed pump power. The inset shows the power stability of the laser output power at 60 mW for 40 min.

The laser linewidth was measured at a laser output power of 100 mW using the self-heterodyne method performed with a 3 km delay fiber (SMF-28M, Corning). Figure 6(a)shows the measured heterodyne signal which was fitted with a Lorentz lineshape. It can be observed that the signal is 90 kHz at 20 dB from the peak, indicating that the fiber laser has a linewidth of 4.5 kHz. Laser noise is an important parameter for a single-frequency fiber laser. Figure 6(b) shows the output RIN results under different laser output powers in the frequency range 0 MHz–15 MHz. The relaxation oscillation frequency peaks under different laser output powers were observed at frequencies of 0.55 MHz,0.95 MHz,and 1.24 MHz,respectively. The relaxation oscillation frequency peaks move toward the higher frequency from 0.55 MHz to 1.24 MHz with increasing output power. The measured RIN is less than?140 dB·Hz?1at frequencies above 10 MHz. Table 2 summarizes the performance of different single-frequency DBR fiber lasers based on RE ion-doped silica glass fiber and YAGderived all-glass fibers. Here, the slope efficiency is defined as the slope of the curve obtained by plotting the laser output power versus the absorbed pump power. It can be found that the output power and the slope efficiency achieved in this work are higher than that in the single-frequency DBR Tm3+doped silica fiber laser.[15]In addition, compared with the other single-frequency DBR YAG-derived all-glass fiber lasers,the performance of the 1.95μm single-frequency DBR fiber laser achieved in this work is competitive. Further improvement should be made with respect to cavity design,such as optimizing the gain fiber numerical aperture(NA)and using high-NA FBGs to optimize the coupling efficiency of pump light.

Fig.6. (a)Linewidth of the single-frequency fiber laser measured by the self-heterodyne method. (b)RIN of the single-frequency fiber laser in the frequency band of 0 MHz–15 MHz with different output powers.

Table 2. Performance of different single-frequency DBR fiber lasers based on RE ion-doped silica fiber and YAG-derived all-glass fibers.

4. Conclusion

In conclusion, a 1.95 μm single-frequency DBR fiber laser was realized by using a 2 cm long Tm:YAG ceramicderived all-glass fiber pumped by a 1610 nm fiber laser. A maximum output power of 135 mW was obtained in this allfiber integrated laser system with a linewidth of 4.5 kHz. The fiber laser has a high OSNR of～77 dB and a low pump threshold of～15.4 mW.In addition,the RIN was investigated under different laser output powers.These results indicate that high-gain Tm:YAG ceramic-derived all-glass fiber is a promising candidate in 2μm single-frequency DBR fiber lasers.

Acknowledgments

Project supported by the Yunnan Fundamental Research Projects (Grant No. 202201AU070065), Natural Science Foundation of China for Young Scholars (Grant No. 52002131), Open Fund of the Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques(Grant No.2021-04),and the Scientific Research Fund Project of Yunnan Provincial Department of Education(Grant No.2022J0591).